45 research outputs found
Determination of step--edge barriers to interlayer transport from surface morphology during the initial stages of homoepitaxial growth
We use analytic formulae obtained from a simple model of crystal growth by
molecular--beam epitaxy to determine step--edge barriers to interlayer
transport. The method is based on information about the surface morphology at
the onset of nucleation on top of first--layer islands in the submonolayer
coverage regime of homoepitaxial growth. The formulae are tested using kinetic
Monte Carlo simulations of a solid--on--solid model and applied to estimate
step--edge barriers from scanning--tunneling microscopy data on initial stages
of Fe(001), Pt(111), and Ag(111) homoepitaxy.Comment: 4 pages, a Postscript file, uuencoded and compressed. Physical Review
B, Rapid Communications, in press
The process of irreversible nucleation in multilayer growth. I. Failure of the mean-field approach
The formation of stable dimers on top of terraces during epitaxial growth is
investigated in detail. In this paper we focus on mean-field theory, the
standard approach to study nucleation. Such theory is shown to be unsuitable
for the present problem, because it is equivalent to considering adatoms as
independent diffusing particles. This leads to an overestimate of the correct
nucleation rate by a factor N, which has a direct physical meaning: in average,
a visited lattice site is visited N times by a diffusing adatom. The dependence
of N on the size of the terrace and on the strength of step-edge barriers is
derived from well known results for random walks. The spatial distribution of
nucleation events is shown to be different from the mean-field prediction, for
the same physical reason. In the following paper we develop an exact treatment
of the problem.Comment: 19 pages, 3 figures. To appear in Phys. Rev.
The role of symmetry on interface states in magnetic tunnel junctions
When an electron tunnels from a metal into the barrier in a magnetic tunnel
junction it has to cross the interface. Deep in the metal the eigenstates for
the electron can be labelled by the point symmetry group of the bulk but around
the interface this symmetry is reduced and one has to use linear combinations
of the bulk states to form the eigenstates labelled by the irreducible
representations of the point symmetry group of the interface. In this way there
can be states localized at the interface which control tunneling. The
conclusions as to which are the dominant tunneling states are different from
that conventionally found.Comment: 14 pages, 5 figures, accepted in PRB, v2: reference 3 complete
Irreversible nucleation in molecular beam epitaxy: From theory to experiments
Recently, the nucleation rate on top of a terrace during the irreversible
growth of a crystal surface by MBE has been determined exactly. In this paper
we go beyond the standard model usually employed to study the nucleation
process, and we analyze the qualitative and quantitative consequences of two
important additional physical ingredients: the nonuniformity of the
Ehrlich-Schwoebel barrier at the step-edge, because of the existence of kinks,
and the steering effects, due to the interaction between the atoms of the flux
and the substrate. We apply our results to typical experiments of second layer
nucleation.Comment: 11 pages. Table I corrected and one appendix added. To be published
in Phys. Rev. B (scheduled issue: 15 February 2003
Structure of self-organized Fe clusters grown on Au(111) analyzed by Grazing Incidence X-Ray Diffraction
We report a detailed investigation of the first stages of the growth of
self-organized Fe clusters on the reconstructed Au(111) surface by grazing
incidence X-ray diffraction. Below one monolayer coverage, the Fe clusters are
in "local epitaxy" whereas the subsequent layers adopt first a strained fcc
lattice and then a partly relaxed bcc(110) phase in a Kurdjumov-Sachs epitaxial
relationship. The structural evolution is discussed in relation with the
magnetic properties of the Fe clusters.Comment: 7 pages, 6 figures, submitted to Physical Review B September 200
Investigation of Single Boron Acceptors at the Cleaved Si:B (111) Surface
The cleaved and (2 x 1) reconstructed (111) surface of p-type Si is
investigated by scanning tunneling microscopy (STM). Single B acceptors are
identified due to their characteristic voltage-dependent contrast which is
explained by a local energetic shift of the electronic density of states caused
by the Coulomb potential of the negatively charged acceptor. In addition,
detailed analysis of the STM images shows that apparently one orbital is
missing at the B site at sample voltages of 0.4 - 0.6 V, corresponding to the
absence of a localized dangling-bond state. Scanning tunneling spectroscopy
confirms a strongly altered density of states at the B atom due to the
different electronic structure of B compared to Si.Comment: 6 pages, 7 figure
Coarsening of Surface Structures in Unstable Epitaxial Growth
We study unstable epitaxy on singular surfaces using continuum equations with
a prescribed slope-dependent surface current. We derive scaling relations for
the late stage of growth, where power law coarsening of the mound morphology is
observed. For the lateral size of mounds we obtain with . An analytic treatment within a self-consistent mean-field
approximation predicts multiscaling of the height-height correlation function,
while the direct numerical solution of the continuum equation shows
conventional scaling with z=4, independent of the shape of the surface current.Comment: 15 pages, Latex. Submitted to PR
Reversed anisotropies and thermal contraction of FCC (110) surfaces
The observed anisotropies of surface vibrations for unreconstructed FCC metal
(110) surfaces are often reversed from the "common sense" expectation. The
source of these reversals is investigated by performing ab initio density
functional theory calculations to obtain the surface force constant tensors for
Ag(110), Cu(110) and Al(110). The most striking result is a large enhancement
in the coupling between the first and third layers of the relaxed surface,
which strongly reduces the amplitude of out-of-plane vibrations of atoms in the
first layer. This also provides a simple explanation for the thermal
contraction of interlayer distances. Both the anisotropies and the thermal
contraction arise primarily as a result of the bond topology, with all three
(110) surfaces showing similar behavior.Comment: 13 pages, in revtex format, plus 1 postscript figur
Fast coarsening in unstable epitaxy with desorption
Homoepitaxial growth is unstable towards the formation of pyramidal mounds
when interlayer transport is reduced due to activation barriers to hopping at
step edges. Simulations of a lattice model and a continuum equation show that a
small amount of desorption dramatically speeds up the coarsening of the mound
array, leading to coarsening exponents between 1/3 and 1/2. The underlying
mechanism is the faster growth of larger mounds due to their lower evaporation
rate.Comment: 4 pages, 4 PostScript figure
Quantum Dimensional Zeeman Effect in the Magneto-optical Absorption Spectrum for Quantum Dot - Impurity Center Systems
Magneto-optical properties of the quantum dot - impurity center (QD-IC)
systems synthesized in a transparent dielectric matrix are considered. For the
QD one-electron state description the parabolic model of the confinement
potential is used. Within the framework of zero-range potential model and the
effective mass approach, the light impurity absorption coefficient for the case
of transversal polarization with respect to the applied magnetic field
direction, with consideration of the QD size dispersion, has been analytically
calculated. It is shown that for the case of transversal polarization the light
impurity absorption spectrum is characterized by the quantum dimensional Zeeman
effect.Comment: 18 pages, 1 figure, PDF fil